Science Bulletin: Electron-plasmon interaction induced plasmonic-polaron bandreplication in epitaxial perovskite SrIrO3 films
发布时间:2020-11-23 作者:Zhengtai Liua,b, Wanling Liua,b,c, Ruixiang Zhouc, Songhua Caid,e, Yekai Songa,b,c, Qi Yaoc, Xiangle Lua,b,Jishan Liua,b, Zhonghao Liua,b, Zhen Wange,f, Yi Zhenge,f, Peng Wangd,e, Zhi Liua,c, Gang Lic,?,Dawei Shena,b,?
https://doi.org/10.1016/j.scib.2020.10.003
Electron-boson interaction is fundamental to a thorough understanding of various exotic propertiesemerging in many-body physics. In photoemission spectroscopy, photoelectron emission due to photonabsorption would trigger diverse collective excitations in solids, including the emergence of phonons,magnons, electron-hole pairs, and plasmons, which naturally provides a reliable pathway to studyelectron-boson couplings. While fingerprints of electron–phonon/-magnon interactions in this state-of-the-art technique have been well investigated, much less is known about electron-plasmon coupling,and direct observation of the band renormalization solely due to electron-plasmon interactions isextremely challenging. Here by utilizing integrated oxide molecular-beam epitaxy and angle-resolvedphotoemission spectroscopy, we discover the long sought-after pure electron-plasmon coupling-induced low-lying plasmonic-polaron replica bands in epitaxial semimetallic SrIrO3films, in which thecharacteristic low carrier concentration and narrow bandwidth combine to provide a unique platformwhere the electron-plasmon interaction can be investigated kinematically in photoemission spec-troscopy. This finding enriches the forms of electron band normalization on collective modes in solidsand demonstrates that, to obtain a complete understanding of the quasiparticle dynamics in 5delectronsystems, the electron-plasmon interaction should be considered on equal footing with the acknowledgedelectron–electron interaction and spin–orbit coupling.
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